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Ultrafast laser systems, those with a pulse duration on the order of picoseconds or less, have enabled advancements in a wide variety of fields. Of particular interest to this work, these laser systems are the key component to many High Energy Density (HED) physics experiments. Despite this, previous studies on the shape of the laser pulse within the HED community have focused primarily on pulse duration due to the relationship between pulse duration and peak intensity, while leaving the femtosecond scale structure of the pulse shape largely unstudied. To broaden the variety of potential pulses available for study, a method of reliably adjusting the pulse shape at the femtosecond scale using sub-nanometer resolution Direct Phase Control has been developed. This paper examines the capabilities of this new method compared to more commonplace dispersion-based pulse shaping methods. It also will detail the capabilities of the core algorithm driving this technique when used in conjunction with the WIZZLER and DAZZLER instruments that are common in high intensity laser labs. Performance of the method and instrumentation is examined using data taken with a single shot FROG system. Finally, some discussion is given to possible applications on how the Direct Phase Control pulse shaping technique will be implemented in the future. 

Complex multiscale flows associated with instabilities and turbulence are commonly induced under high-energy density (HED) conditions, but accurate measurement of their transport properties has been challenging. x-ray photon correlation spectroscopy (XPCS) with coherent xx-ray sources can, in principle, probe material dynamics to infer transport properties using time autocorrelation of density fluctuations. Here we develop a theoretical framework for utilizing XPCS to study material diffusivity in multiscale flows. We extend single-scale shear flow theories to broadband flows using a multiscale analysis that captures shear and diffusion dynamics. Our theory is validated with simulated XPCS for Brownian particles advected in multiscale flows. We demonstrate the versatility of the method over several orders of magnitude in timescale using sequential-pulse XPCS, single-pulse xx-ray speckle visibility spectroscopy (XSVS), and double-pulse XSVS. Published by the American Physical Society2025 

Abstract The properties of all materials at one atmosphere of pressure are controlled by the configurations of their valence electrons. At extreme pressures, neighboring atoms approach so close that core-electron orbitals overlap, and theory predicts the emergence of unusual quantum behavior. We ramp-compress monovalent elemental sodium, a prototypical metal at ambient conditions, to nearly 500 GPa (5 million atmospheres). The 7-fold increase of density brings the interatomic distance to 1.74 Å well within the initial 2.03 Å of the Na + ionic diameter, and squeezes the valence electrons into the interstitial voids suggesting the formation of an electride phase. The laser-driven compression results in pressure-driven melting and recrystallization in a billionth of a second. In situ x-ray diffraction reveals a series of unexpected phase transitions upon recrystallization, and optical reflectivity measurements show a precipitous decrease throughout the liquid and solid phases, where the liquid is predicted to have electronic localization. These data reveal the presence of a rich, temperature-driven polymorphism where core electron overlap is thought to stabilize the formation of peculiar electride states. 

The discovery of more than 4500 extrasolar planets has created a need for modeling their interior structure and dynamics. Given the prominence of iron in planetary interiors, we require accurate and precise physical properties at extreme pressure and temperature. A first-order property of iron is its melting point, which is still debated for the conditions of Earth’s interior. We used high-energy lasers at the National Ignition Facility and in situ x-ray diffraction to determine the melting point of iron up to 1000 gigapascals, three times the pressure of Earth’s inner core. We used this melting curve to determine the length of dynamo action during core solidification to the hexagonal close-packed (hcp) structure. We find that terrestrial exoplanets with four to six times Earth’s mass have the longest dynamos, which provide important shielding against cosmic radiation.